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Phys. Rev. Lett. 100, 137202 (2008) [4 pages]

Field-Dependent Thermal Transport in the Haldane Chain Compound NENP

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A. V. Sologubenko1, T. Lorenz1, J. A. Mydosh1, A. Rosch2, K. C. Shortsleeves3, and M. M. Turnbull3
1II. Physikalisches Institut, Universität zu Köln, 50937 Köln, Germany
2Institut für Theoretische Physik, Universität zu Köln, 50937 Köln, Germany
3Carlson School of Chemistry and Biochemistry, Clark University, Worcester, Massachusetts 01610, USA

Received 24 December 2007; revised 6 February 2008; published 2 April 2008

We present a study of the magnetic field-dependent thermal transport in the spin S=1 chain material Ni(C2H8N2)2NO2(ClO4) (NENP). The measured thermal conductivity is found to be very sensitive to the field-induced changes in the spin excitation spectrum. The magnetic contribution to the total heat conductivity is analyzed in terms of a quasiparticle model, and we obtain a temperature and momentum independent mean free path. This implies that the motion of quasiparticles is effectively three dimensional despite the tiny interchain coupling.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.100.137202
DOI:
10.1103/PhysRevLett.100.137202
PACS:
75.40.Gb, 66.70.−f, 75.47.−m