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Phys. Rev. Lett. 100, 247002 (2008) [4 pages]

Superconductivity at 41 K and Its Competition with Spin-Density-Wave Instability in Layered CeO1-xFxFeAs

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G. F. Chen, Z. Li, D. Wu, G. Li, W. Z. Hu, J. Dong, P. Zheng, J. L. Luo, and N. L. Wang
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, People’s Republic of China

Received 15 April 2008; revised 14 May 2008; published 16 June 2008

A series of layered CeO1-xFxFeAs compounds with x=0 to 0.20 are synthesized by the solid state reaction method. Similar to the LaOFeAs, the pure CeOFeAs shows a strong resistivity anomaly near 145 K, which was ascribed to the spin-density-wave instability. F doping suppresses this instability and leads to the superconducting ground state. Most surprisingly, the superconducting transition temperature could reach as high as 41 K. Such a high Tc strongly challenges the classic BCS theory based on the electron-phonon interaction. The closeness of the superconducting phase to the spin-density-wave instability suggests that the magnetic fluctuation plays a key role in the superconducting pairing mechanism. The study also reveals that the Ce 4f electrons form local moments and are ordered antiferromagnetically below 4 K, which could coexist with superconductivity.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.100.247002
DOI:
10.1103/PhysRevLett.100.247002
PACS:
74.70.−b, 74.25.Gz, 74.62.Bf