corner
corner

Phys. Rev. Lett. 100, 056401 (2008) [4 pages]

Coherent and Incoherent Excitations of Electron-Doped SrTiO3

Download: PDF (759 kB) Buy this article Export: BibTeX or EndNote (RIS)

Yukiaki Ishida1, Ritsuko Eguchi1, Masaharu Matsunami1, Koji Horiba1, Munetaka Taguchi1, Ashish Chainani1, Yasunori Senba2, Haruhiko Ohashi2, Hiromichi Ohta3, and Shik Shin1,4
1RIKEN SPring-8 Center, Sayo, Sayo, Hyogo 679-5148, Japan
2JASRI/SPring-8, Sayo, Sayo, Hyogo 679-5198, Japan
3Graduate School of Engineering, Nagoya University, Furo, Chikusa, Nagoya, Aichi 464-8603, Japan
4ISSP, University of Tokyo, Kashiwa-no-ha, Kashiwa, Chiba 277-8561, Japan

Received 19 February 2007; published 4 February 2008

Resonant photoemission at the Ti 2p and O 1s edges on a Nb-doped SrTiO3 thin film revealed that the coherent state (CS) at the Fermi level (EF) had a mainly Ti 3d character whereas the incoherent in-gap state (IGS) positioned ∼1.5  eV below EF had a mixed character of Ti 3d and O 2p states. This indicates that the IGS is formed by a spectral-weight transfer from the CS and subsequent spectral-weight redistribution through d-p hybridization. We discuss the evolution of the excitation spectrum with 3d band filling and rationalize the IGS through a mechanism similar to that proposed by Haldane and Anderson.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.100.056401
DOI:
10.1103/PhysRevLett.100.056401
PACS:
71.28.+d, 71.10.−w, 79.60.−i