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Phys. Rev. Lett. 101, 116401 (2008) [4 pages]

Strong Exciton-Photon Coupling in an Organic Single Crystal Microcavity

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S Kéna-Cohen1,2, M. Davanço2, and S. R. Forrest2,*
1Princeton Institute for the Science and Technology of Materials (PRISM), Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
2Departments of Electrical Engineering and Computer Science and Physics, University of Michigan, Ann Arbor, Michigan 48109, USA

Received 30 March 2008; revised 11 July 2008; published 9 September 2008

We demonstrate strong exciton-photon coupling of Frenkel excitons at room temperature in a microcavity composed of a melt grown thin film anthracene single crystal and two distributed Bragg reflectors. Angle-resolved reflectivity and normal incidence photoluminescence under weak excitation are observed. The microcavity spectrum is a function of the anisotropy of the crystalline material and the strong exciton-photon coupling of the excitonic resonances to the cavity photon. The photoluminescence spectrum is found to be completely polarized along the crystal axes.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.101.116401
DOI:
10.1103/PhysRevLett.101.116401
PACS:
71.36.+c, 78.66.Qn

*To whom correspondence should be addressed.

stevefor@umich.edu