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Phys. Rev. Lett. 101, 217201 (2008) [4 pages]

Spin-Electric Coupling in Molecular Magnets

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Mircea Trif1, Filippo Troiani2, Dimitrije Stepanenko1, and Daniel Loss1
1Department of Physics, University of Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland
2CNR-INFM National Research Center S3 c/o Dipartimento di Fisica via G. Campi 213/A, 41100, Modena, Italy

Received 8 May 2008; published 20 November 2008

We study the triangular antiferromagnet Cu3 in external electric fields, using symmetry group arguments and a Hubbard model approach. We identify a spin-electric coupling caused by an interplay between spin exchange, spin-orbit interaction, and the chirality of the underlying spin texture of the molecular magnet. This coupling allows for the electric control of the spin (qubit) states, e.g., by using an STM tip or a microwave cavity. We propose an experimental test for identifying molecular magnets exhibiting spin-electric effects.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.101.217201
DOI:
10.1103/PhysRevLett.101.217201
PACS:
75.50.Xx, 03.67.Lx