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Phys. Rev. Lett. 101, 073003 (2008) [4 pages]

Recoil-Ion Momentum Distributions for Two-Photon Double Ionization of He and Ne by 44 eV Free-Electron Laser Radiation

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A. Rudenko1,2, L. Foucar3, M. Kurka2, Th. Ergler2, K. U. Kühnel2, Y. H. Jiang2, A. Voitkiv2, B. Najjari2, A. Kheifets4, S. Lüdemann2, T. Havermeier3, M. Smolarski3, S. Schössler3, K. Cole3, M. Schöffler3, R. Dörner3, S. Düsterer5, W. Li5, B. Keitel5, R. Treusch5, M. Gensch5, C. D. Schröter2, R. Moshammer1,2, and J. Ullrich1,2
1Max-Planck Advanced Study Group at CFEL, Notkestrasse 85, 22607 Hamburg, Germany
2Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany
3Institut für Kernphysik, Universität Frankfurt, 60486 Frankfurt, Germany
4Research School of Physical Sciences, The Australian University, Canberra, ACT 0200, Australia
5DESY, Notkestrasse 85, 22607 Hamburg, Germany

Received 12 February 2008; published 15 August 2008

Recoil-ion momentum distributions for two-photon double ionization of He and Ne (ω=44  eV) have been recorded with a reaction microscope at FLASH (the free-electron laser at Hamburg) at an intensity of ∼1×1014  W/cm2 exploring the dynamics of the two fundamental two-photon–two-electron reaction pathways, namely, sequential and direct (or nonsequential) absorption of the photons. We find strong differences in the recoil-ion momentum patterns for the two mechanisms pointing to the significantly different two-electron emission dynamics and thus provide serious constraints for theoretical models.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.101.073003
DOI:
10.1103/PhysRevLett.101.073003
PACS:
32.80.Rm, 41.60.Cr, 42.65.−k