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Phys. Rev. Lett. 102, 127404 (2009) [4 pages]

Gain Control in Semiconductor Quantum Dots via State-Resolved Optical Pumping

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Ryan R. Cooney, Samuel L. Sewall, D. M. Sagar, and Patanjali Kambhampati*
Department of Chemistry, McGill University, Montreal, QC, H3A 2K6, Canada

Received 28 October 2008; published 24 March 2009

Excitonic state-resolved optical pumping experiments were performed on strongly confined semiconductor quantum dots. We demonstrate for the first time that optical gain is dependent upon the initial excitonic state. By prescribing the specific multiexcitonic states which can create, block, and ultimately control optical gain spectra, we recover the theoretically predicted size independence, even in systems which previously showed zero gain. In addition, we show for the first time that stimulated emission in quantum dots can be controlled via specific multiexcitonic interactions.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.102.127404
DOI:
10.1103/PhysRevLett.102.127404
PACS:
78.67.Hc, 73.21.La, 78.45.+h, 82.53.Mj

*To whom all correspondence should be addressed.

pat.kambhampati@mcgill.ca.