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Phys. Rev. Lett. 102, 207205 (2009) [4 pages]

Flop of Electric Polarization Driven by the Flop of the Mn Spin Cycloid in Multiferroic TbMnO3

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N. Aliouane1,2, K. Schmalzl3, D. Senff4, A. Maljuk1, K. Prokeš1, M. Braden4, and D. N. Argyriou1,*
1Helmholtz-Zentrum Berlin für Materialen und Energy, Glienicker Straße 100, D-14109 Berlin, Germany
2Institute For Energy Technology, Post Office Box 40, NO-2027 Kjeller, Norway
3Institut für Festkörperforschung, Forschungszentrum Jülich GmbH, JCNS at ILL, 38042 Grenoble Cedex 9, France
4II. Physikalisches Institut, Universität zu Köln, Zülpicher Straße 77, D-50937 Köln, Germany

Received 11 February 2009; published 20 May 2009

Using in-field single-crystal neutron diffraction, we have determined the magnetic structure of TbMnO3 in the high field Pa phase. We unambiguously establish that the ferroelectric polarization arises from a cycloidal Mn spin ordering, with spins rotating in the ab plane. Our results demonstrate directly that the flop of the ferroelectric polarization in TbMnO3 with applied magnetic field is caused from the flop of the Mn cycloidal plane.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.102.207205
DOI:
10.1103/PhysRevLett.102.207205
PACS:
75.25.+z, 61.05.F−, 75.10.−b, 75.30.Et

*argyriou@helmholtz-berlin.de