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Phys. Rev. Lett. 102, 096403 (2009) [4 pages]

Quantized Hyperfine Field at an Implanted μ+ Site in PrPb3: Interplay between Localized f Electrons and an Interstitial Charged Particle

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T. U. Ito1,2, W. Higemoto2, K. Ohishi2,*, N. Nishida1, R. H. Heffner2,3, Y. Aoki4, A. Amato5, T. Onimaru6, and H. S. Suzuki7
1Department of Physics, Tokyo Institute of Technology, Meguro, Tokyo 152-8551, Japan
2Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195, Japan
3Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
4Department of Physics, Tokyo Metropolitan University, Hachioji, Tokyo 192-0397, Japan
5Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
6Department of Quantum Matter, ADSM, Hiroshima University, Higashi-Hiroshima, Hiroshima 739-8530, Japan
7National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan

Received 28 October 2008; published 3 March 2009

The local effect of an interstitial hydrogenlike particle on localized f electrons was studied in PrPb3 by means of μ+ spin rotation and relaxation. Spontaneous μ+ spin precession with harmonic frequencies was observed for the first time in f electron compounds. We demonstrate that the signal is derived from a coupling between the μ+ spin and the hyperfine-enhanced nuclear spin of nearest neighbor (NN) 141Pr with Ising-like anisotropy. The signal also suggests a marked suppression of spin dynamics of the NN 141Pr in comparison with that of the bulk 141Pr. These facts strongly indicate modification of the f electronic state due to the interstitial charged particle.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.102.096403
DOI:
10.1103/PhysRevLett.102.096403
PACS:
71.70.Ch, 76.75.+i

*Present address: Advanced Meson Science Laboratory, RIKEN, Wako 351-0198, Japan.