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Phys. Rev. Lett. 103, 176601 (2009) [4 pages]

Efficient Spin Transitions in Inelastic Electron Tunneling Spectroscopy

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Nicolás Lorente1 and Jean-Pierre Gauyacq2,3
1Centre d’Investigació en Nanociència i Nanotecnologia (CSIC-ICN), Campus de la UAB, Bellaterra, Spain
2CNRS, Laboratoire des Collisions Atomiques et Moléculaires, UMR 8625, Bât.351, 91405 Orsay, France
3Université Paris-Sud, Laboratoire des Collisions Atomiques et Moléculaires, UMR 8625, Bât.351, 91405 Orsay, France

Received 28 April 2009; published 21 October 2009

The excitation of the spin degrees of freedom of an adsorbed atom by tunneling electrons is computed using strong coupling theory. Recent measurements [ Heinrich et al. Science 306 466 (2004)] reveal that electron currents in a magnetic system efficiently excite its magnetic moments. Our theory shows that the incoming electron spin strongly couples with that of the adsorbate so that memory of the initial spin state is lost, leading to large excitation efficiencies. First-principles transmissions are evaluated in quantitative agreement with the experiment.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.103.176601
DOI:
10.1103/PhysRevLett.103.176601
PACS:
72.25.−b, 68.37.Ef, 72.10.−d, 73.23.−b