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Phys. Rev. Lett. 103, 197401 (2009) [4 pages]

Direct Observation of the Critical Relaxation of Polarization Clusters in BaTiO3 Using a Pulsed X-Ray Laser Technique

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K. Namikawa1,2,6, M. Kishimoto2,6, K. Nasu3,6, E. Matsushita4,6, R. Z. Tai5,6, K. Sukegawa2, H. Yamatani2, H. Hasegawa2, M. Nishikino2, M. Tanaka2,6, and K. Nagashima2
1Department of Physics, Tokyo Gakugei University, Koganei, Tokyo 184-8501, Japan
2Quantum Beam Science Directorate, Japan Atomic Energy Agency, Kizugawa, Kyoto 619-0215, Japan
3IMSS, KEK, Tsukuba, Ibaraki 305-0801, Japan
4Faculty of Engineering, Gifu University, Gifu, Gifu 501-1193, Japan
5Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Science, Shanghai 201204, China
6Japan Science and Technology Agency, CREST, Chiyoda, Tokyo 102-0075, Japan

Received 30 September 2008; revised 24 June 2009; published 5 November 2009

We have developed a new method to investigate the relaxation time of the dipole moment in polarization clusters in BaTiO3. Time correlation of speckle intensities was measured by the use of a double pulsed soft x-ray laser. The evolution of the relaxation time of the dipole moment near the Curie temperature (TC) was investigated. The maximum relaxation time (∼90  ps) is shown to appear at a temperature of 4.5 K above the TC, being coincident with the one where the maximum polarization takes place. This method is widely applicable to any other critical decay processes at phase transitions.

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© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.103.197401
DOI:
10.1103/PhysRevLett.103.197401
PACS:
78.70.Ck, 61.05.cf, 77.80.Bh, 77.84.Dy