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Phys. Rev. Lett. 103, 047403 (2009) [4 pages]

Nonequilibrium Steady State of Photoexcited Correlated Electrons in the Presence of Dissipation

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Naoto Tsuji, Takashi Oka, and Hideo Aoki
Department of Physics, University of Tokyo, Hongo, Tokyo 113-0033, Japan

Received 13 March 2009; published 24 July 2009

We present a framework to determine nonequilibrium steady states in strongly correlated electron systems in the presence of dissipation. This is demonstrated for a correlated electron (Falicov-Kimball) model attached to a heat bath and irradiated by an intense pump light, for which an exact solution is obtained with the Floquet method combined with the nonequilibrium dynamical mean-field theory. On top of a Drude-like peak indicative of photometallization as observed in recent pump-probe experiments, new nonequilibrium phenomena are predicted to emerge, where the optical conductivity exhibits dip and kink structures around the frequency of the pump light, a midgap absorption arising from photoinduced Floquet subbands, and a negative attenuation (gain) due to a population inversion.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.103.047403
DOI:
10.1103/PhysRevLett.103.047403
PACS:
78.20.Bh, 05.30.Fk, 71.27.+a, 78.47.−p