Phys. Rev. Lett. 44, 139–142 (1980)Two-Photon Technique for the Dissociative Spectroscopy of Simple MoleculesReceived 15 June 1979; published in the issue dated 21 January 1980 A two-photon technique is reported for the measurement of relative cross sections for the photolysis of simple molecules into particular product channels. In a demonstration of this method, two independently tunable dye lasers were used to dissociate molecules of Cs2 sequentially for wavelengths in the range 445 to 505 nm, and then to excite the resulting products to determine the relative cross sections for the photolysis of the Cs2 molecules into each of the energetically possible product states. © 1980 The American Physical Society URL:
http://link.aps.org/doi/10.1103/PhysRevLett.44.139
DOI:
10.1103/PhysRevLett.44.139
PACS:
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