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Phys. Rev. Lett. 73, 189–192 (1994)

Magnetic structure of the spin-liquid state in a frustrated pyrochlore

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M. J. Harris, M. P. Zinkin, Z. Tun, B. M. Wanklyn, and I. P. Swainson
Oxford Physics, Clarendon Laboratory, Parks Road, Oxford, OX1 3PU, United Kingdom
Neutron and Condensed Matter Science, AECL Research, Chalk River Laboratories, Chalk River, Ontario, Canada, K0J 1J0

Received 10 February 1994; published in the issue dated 4 July 1994

The antiferromagnetic pyrochlores exhibit a high degree of frustration, resulting in a continuously disordered ground state. Neutron powder diffraction experiments have detected magnetic scattering similar in form to a liquid structure factor. We present a single crystal neutron scattering study of the pyrochlore CsNiCrF6 and quantify the anisotropy of the scattering. Using these data, we show that there are strong correlations between nearest-neighbor spins, and no significant longer correlations. This provides clear evidence for the liquidlike nature of the pyrochlore magnetic structure.

© 1994 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.73.189
DOI:
10.1103/PhysRevLett.73.189
PACS:
75.50.Lk, 75.25.+z, 75.40.Gb