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Phys. Rev. Lett. 75, 4702–4705 (1995)

Electron Dynamics in Copper Metallic Nanoparticles Probed with Femtosecond Optical Pulses

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J. -Y. Bigot, J. -Y. Merle, O. Cregut, and A. Daunois
Insitut de Physique et Chimie des Matériaux de Strasbourg, Groupe d'Optique Nonlinéaire et d'Optoélectronique, Unité mixte 380046 CNRS-ULP-EHICS, 23 rue du Loess, 67037 Strasbourg Cedex, France

Received 9 May 1995; published in the issue dated 18 December 1995

The thermalization of electrons in copper nanoparticles embedded in glass is investigated using femtosecond pump-probe spectroscopy. The time dependent induced transmission is enhanced near the surface plasmon resonance of the nanoparticles, as opposed to the static one obtained with thermomodulation measurements. In addition, a slowing of the process of electron cooling to the lattice temperature is observed at the plasmon resonance. These observations show the importance of quasiparticle collisions in confined metallic structures.

© 1995 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.75.4702
DOI:
10.1103/PhysRevLett.75.4702
PACS:
78.47.+p