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Phys. Rev. Lett. 76, 2125–2128 (1996)

Spin Fluctuations in (Y0.97Sc0.03)Mn2: A Geometrically Frustrated, Nearly Antiferromagnetic, Itinerant Electron System

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R. Ballou
Laboratoire de Magnétisme Louis Néel–CNRS, BP 166, 38042 Grenoble Cedex 9, France

E. Lelièvre-Berna
Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9, France

B. Fåk
Commissariat à l'Energie de Physique Theorique, Département de Recherche Fondamentale sur la Matière Condensée, SPSMS/MDN, 17 rue des Martyrs, 38054 Grenoble Cedex 9, France

See Also: Erratum

Received 8 August 1995; published in the issue dated 18 March 1996

Inelastic neutron-scattering experiments have been performed on a single crystal of (Y0.97Sc0.03)Mn2. The spin fluctuation spectrum is broad in energy and strongly correlated in wave vector, with maximum intensity at the Brillouin zone boundary. There is no magnetic scattering for Brillouin zones centered at the origin and at certain reciprocal lattice points, suggesting the existence of short-lived 4-site collective spin singlets. The unusual features of the dynamical susceptibility discovered in this experiment result from geometrical frustration and give new insight into the heavy-fermion-like behavior of the compound.

© 1996 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.76.2125
DOI:
10.1103/PhysRevLett.76.2125
PACS:
71.27.+a, 75.40.Gb, 75.50.Ee

See Also

Erratum: R. Ballou, E. Lelièvre-Berna, and B. Fåk, Spin Fluctuations in (Y0.97Sc0.03)Mn2: A Geometrically Frustrated, Nearly Antiferromagnetic, Itinerant Electron System, Phys. Rev. Lett. 77, 790 (1996).