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Phys. Rev. Lett. 77, 3661–3664 (1996)

Coherent THz Phonons Driven by Light Pulses and the Sb Problem: What is the Mechanism?

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G. A. Garrett1,2, T. F. Albrecht1,2, J. F. Whitaker1, and R. Merlin1,2,3
1Center for Ultrafast Optical Science, The University of Michigan, Ann Arbor, Michigan 48109-2099
2The Harrison M. Randall Laboratory of Physics, The University of Michigan, Ann Arbor, Michigan 48109-1120
3Department of Physics, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong

Received 23 July 1996; published in the issue dated 21 October 1996

Femtosecond laser pulses generate in Sb coherent Eg phonons at 3.4 THz, in addition to oscillations of A1g symmetry accounted for by the phenomenological displacive-excitation model. Experiments agree with theoretical calculations showing that the coherent driving force in absorbing materials like Sb is determined by Raman processes, as in transparent media. The Raman formalism provides a unifying approach for describing light-induced motion of atoms of both impulsive and displacive character.

© 1996 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.77.3661
DOI:
10.1103/PhysRevLett.77.3661
PACS:
78.47.+p, 63.20.Kr, 78.30.-j