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Phys. Rev. Lett. 80, 2713–2716 (1998)

Nuclear Magnetic Resonance Study of the S = 1/2 Heisenberg Ladder Cu2(C5H12N2)2Cl4: Quantum Phase Transition and Critical Dynamics

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G. Chaboussant1, Y. Fagot-Revurat1, M.-H. Julien1, M. E. Hanson1, C. Berthier1,3, M. Horvatić1, L. P. Lévy1,2, and O. Piovesana4
1Grenoble High Magnetic Field Laboratory, CNRS and MPI-FKF, B.P. 166, 38042 Grenoble Cedex 09, France
2Institut Universitaire de France and Université J. Fourier, B.P. 41, F-38400 St. Martin d'Hères, France
3Laboratoire de Spectrométrie Physique, Université J. Fourier, B.P. 87, F-38402 St. Martin d'Hères, France
4Dipartimento di Chimica, Universitá di Perugia, I-06100 Perugia, Italy

Received 12 August 1997; published in the issue dated 23 March 1998

We present an extensive NMR study of the spin-1/2 antiferromagnetic Heisenberg ladder Cu2(C5H12N2)2Cl4 in a magnetic field range 4.5–16.7 T. By measuring the proton NMR relaxation rate 1/T1 and varying the magnetic field around the critical field Hc1 = Δ/gμB7.5T, we have studied the transition from a gapped spin liquid ground state to a gapless magnetic regime which can be described as a Luttinger liquid. We identify an intermediate regime T|H-Hc1|, where the spin dynamics is (possibly) only controlled by the T = 0 critical point Hc1.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.80.2713
DOI:
10.1103/PhysRevLett.80.2713
PACS:
75.10.Jm, 75.40.Cx, 76.60.-k