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Phys. Rev. Lett. 80, 5077–5080 (1998)

Local-Field Effects on Spontaneous Emission in a Dense Supercritical Gas

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Frank J. P. Schuurmans, Dennis T. N. de Lang, Gerard H. Wegdam, Rudolf Sprik, and Ad Lagendijk
Van der Waals-Zeeman Instituut, Universiteit van Amsterdam, Valckenierstraat 65, 1018 XE Amsterdam, The Netherlands

Received 9 January 1998; published in the issue dated 8 June 1998

We present results of experiments on the spontaneous emission rate of a europium complex in dense supercritical CO2. The refractive index of the supercritical gas is varied from 1.00 to 1.27 by increasing the pressure up to a 1000 bars. Accordingly, the spontaneous emission rate changes. Local-field effects on spontaneous emission are clearly observed in these experiments. The empty-cavity model for the spontaneous emission rate inside dielectrics is confirmed.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.80.5077
DOI:
10.1103/PhysRevLett.80.5077
PACS:
32.80.-t, 42.50.-p, 78.55.-m