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Phys. Rev. Lett. 80, 604–607 (1998)

NMR Study of Zn Doping Effect in Spin Ladder System SrCu2O3

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N. Fujiwara* and H. Yasuoka
Institute for Solid State Physics, University of Tokyo, Roppongi, Minato-ku, Tokyo 106, Japan

Y. Fujishiro, M. Azuma, and M. Takano
Institute for Chemistry, Kyoto University, Uji, Kyoto-fu 611, Japan

Received 16 June 1997; published in the issue dated 19 January 1998

Nuclear magnetic resonance spectra of Cu nuclei were measured in a typical spin ladder system, Sr(Cu1-xZnx)2O3 ( x = 0%, 0.25%, and 0.5%) at temperatures ranging from room temperature to 20 K. The linewidth of the spectrum peaks drastically increased at temperatures below 100 K with x being only 0.25%. The width ΔW increased with the increase in Zn concentration and the decrease in temperatures (ΔWx/T). These facts prove that a quite minute amount of impurity breaks the singlet ground state and the effect of impurity is observed in the whole system.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.80.604
DOI:
10.1103/PhysRevLett.80.604
PACS:
75.40.Gb, 76.60.Es

*Electronic address: naokif@ginnan.issp.u-tokyo.ac.jp