Phys. Rev. Lett. 82, 4142–4145 (1999)

Three-Dimensional Vibrational Imaging by Coherent Anti-Stokes Raman Scattering

Abstract

References

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Andreas Zumbusch^*, Gary R. Holtom, and X. Sunney Xie^†
Pacific Northwest National Laboratory, William R. Wiley Environmental Molecular Sciences Laboratory, P.O. Box 999, K8-88, Richland, Washington 99352

Received 9 December 1998; published in the issue dated 17 May 1999

See accompanying Physics Focus

A multiphoton microscopy based on coherent anti-Stokes Raman scattering is accomplished with near-infrared ultrashort laser pulses. We demonstrate vibrational imaging of chemical and biological samples with high sensitivity, high spatial resolution, noninvasiveness, and three-dimensional sectioning capability.

URL:

http://link.aps.org/doi/10.1103/PhysRevLett.82.4142

DOI:

10.1103/PhysRevLett.82.4142

PACS:

87.64.Je, 87.15.Mi, 87.16.Tb, 87.64.Vv

^*Present address: Institute für Physikalische Chemie, Universität München, Butenandtstr. 5-13 Haus E, D-81377 München, Germany.

^†Present address: Harvard University, Department of Chemistry and Chemical Biology, 12 Oxford Street, Cambridge, MA 01238.

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Phys. Rev. Lett. 82, 4142–4145 (1999)

Three-Dimensional Vibrational Imaging by Coherent Anti-Stokes Raman Scattering