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Phys. Rev. Lett. 83, 211–214 (1999)

Glassy Statics and Dynamics in the Chemically Ordered Pyrochlore Antiferromagnet Y2Mo2O7

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J. S. Gardner1, B. D. Gaulin1, S.-H. Lee2, C. Broholm2,3, N. P. Raju4, and J. E. Greedan4
1Department of Physics and Astronomy, McMaster University, Hamilton, Ontario, Canada L8S 4M1
2National Institute of Standards and Technology, Gaithersburg, Maryland 20899
3Department of Physics and Astronomy, The John Hopkins University, Baltimore, Maryland 21218
4Brockhouse Institute for Materials Research, McMaster University, Hamilton, Ontario, Canada L8S 4M1

Received 4 January 1999; published in the issue dated 5 July 1999

Static and dynamic magnetic correlations in the geometrically frustrated pyrochlore antiferromagnet Y2Mo2O7 have been studied using neutron scattering. The material is chemically ordered but displays a spin-freezing transition at Tg22.5 K. We show that dynamic short range order develops below room temperature. Upon cooling the two-spin correlation length never exceeds 5 Å, yet the spin fluctuation rate vanishes in proportion to T-Tg. For T<Tg low energy spin fluctuations are replaced by static antiferromagnetic short range order with a frozen staggered magnetization |S|/S0.67(2). Locally the frozen spin structure corresponds to four sublattice ordering with zero magnetization.

© 1999 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.83.211
DOI:
10.1103/PhysRevLett.83.211
PACS:
75.50.Lk, 75.25.+z, 75.40.Cx, 75.40.Gb