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Phys. Rev. Lett. 83, 4880–4883 (1999)

Infrared Studies of the Onset of Conductivity in Ultrathin Pb Films

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P. F. Henning1,2, C. C. Homes1, S. Maslov1, G. L. Carr1, D. N. Basov2, B. Nikolić3, and M. Strongin1
1Department of Physics, Brookhaven National Laboratory, Upton, New York 11973
2Department of Physics, University of California at San Diego, La Jolla, California 92093
3Department of Physics, SUNY at Stony Brook, Stony Brook, New York 11794

Received 23 April 1999; published in the issue dated 6 December 1999

In this paper we report the first experimental measurement of the low-temperature, normal-state infrared conductivity of ultrathin quenched-condensed Pb films. For dc sheet resistances such that ωτ≪1 the ac conductance increases with frequency but is in disagreement with the predictions of weak localization. We attribute this behavior to the effects of an inhomogeneous granular structure in these films when they are first formed, which is manifested at the very small probing scale of infrared measurements. Our data are consistent with predictions of two-dimensional percolation theory.

© 1999 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.83.4880
DOI:
10.1103/PhysRevLett.83.4880
PACS:
78.66.Bz, 74.76.Db, 72.15.Rn