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Phys. Rev. Lett. 83, 524–527 (1999)

Irregular Orbits Generate Higher Harmonics

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Gerd van de Sand1 and Jan M. Rost1,2a,2b
1Theoretical Quantum Dynamics, Fakultät für Physik, Universität Freiburg, Hermann-Herder-Strasse 3, D-79104 Freiburg, Germany
2aInstitute for Advanced Study, Wallotstrasse 19, D-14193 Berlin, Germany
2band Max-Planck-Institute for Physics of Complex Systems, Nöthnitzer Strasse 38, D-01187 Dresden, Germany

Received 25 March 1999; published in the issue dated 19 July 1999

The spectrum of higher harmonics in atoms calculated with a uniformized semiclassical propagator is presented and it is shown that the higher harmonic generation is an interference phenomenon which can be described semiclassically. This can be concluded from the good agreement with the quantum spectrum. Moreover, the formation of a plateau in the spectrum is specifically due to the interference of irregular, time-delayed, trajectories with regular orbits without a time delay. This is proven by the absence of the plateau in an artificial semiclassical spectrum generated from a sample of trajectories from which the irregular trajectories (only a few percent) have been discarded.

© 1999 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.83.524
DOI:
10.1103/PhysRevLett.83.524
PACS:
32.80.Wr, 03.65.Sq, 05.45.Mt