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Phys. Rev. Lett. 84, 3430–3433 (2000)

Dipolar Interactions and Origin of Spin Ice in Ising Pyrochlore Magnets

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Byron C. den Hertog1 and Michel J. P. Gingras1,2
1Department of Physics, University of Waterloo, Waterloo, Ontario, Canada N2L 3G1
2Canadian Institute for Advanced Research, 180 Dundas Street W, Toronto, Ontario, Canada M5G 1Z8

Received 8 November 1999; published in the issue dated 10 April 2000

Recent experiments suggest that the Ising pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 display qualitative properties of the nearest-neighbor “spin ice” model. We discuss the dipolar energy scale present in both these materials and discuss how spin-ice behavior can occur despite the presence of long-range dipolar interactions. We present results of numerical simulations and a mean field analysis of Ising pyrochlore systems. Based on our quantitative theory, we suggest that the spin-ice behavior in these systems is due to long-range dipolar interactions, and that the nearest-neighbor exchange in Dy2Ti2O7 is antiferromagnetic.

© 2000 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.84.3430
DOI:
10.1103/PhysRevLett.84.3430
PACS:
75.10.Hk, 05.50.+q, 75.30.Kz, 75.40.Mg