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Phys. Rev. Lett. 85, 5428–5431 (2000)

Anisotropic Optical Spectra of PrBa2Cu4O8: Possible Tomonaga-Luttinger Liquid Response of the Quasi-One-Dimensional Metallic CuO Double Chains

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K. Takenaka1,*, K. Nakada2, A. Osuka1, S. Horii3, H. Ikuta4, I. Hirabayashi5, S. Sugai1, and U. Mizutani2
1Department of Physics, Nagoya University, Nagoya 464-8602, Japan
2Department of Crystalline Materials Science, Nagoya University, Nagoya 464-8603, Japan
3Department of Applied Chemistry, University of Tokyo, Tokyo 113-8656, Japan
4Center for Integrated Research in Science and Engineering (CIRSE), Nagoya University, Nagoya 464-8603, Japan
5Superconductivity Research Laboratory, International Superconductivity Technology Center, Nagoya 456-8587, Japan

Received 10 May 2000; published in the issue dated 18 December 2000

The optical spectra of PrBa2Cu4O8 show large in-plane anisotropy. For the a polarization ( E  chain), the spectrum is characterized by a gap of 1.4 eV, indicating the charge-transfer insulating nature of the CuO2 planes. For the metallic chain direction ( Eb), the spectrum deviates from a simple Drude response; reflectivity Rb(ω) shows a sharp edge at 1eV but it also shows a dip at 15meV, which splits the conductivity spectrum into two parts—a zero-energy mode with small weight and a pronounced 40meV mode. These features are discussed in terms of a Tomonaga-Luttinger liquid in a doped 1D Mott insulator and compared with 1D Bechgaard salts.

© 2000 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.85.5428
DOI:
10.1103/PhysRevLett.85.5428
PACS:
78.20.-e, 72.15.-v, 74.72.Jt

*Electronic address: k46291a@nucc.cc.nagoya-u.ac.jp