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Phys. Rev. Lett. 85, 1986–1989 (2000)

Ultrafast Spin Dynamics and Critical Behavior in Half-Metallic Ferromagnet: Sr2FeMoO6

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T. Kise1, T. Ogasawara1, M. Ashida2, Y. Tomioka3, Y. Tokura1,3, and M. Kuwata-Gonokami1,2,*
1Department of Applied Physics, The University of Tokyo, Tokyo 113-8656, Japan
2Cooperative Excitation Project, ERATO, Japan Science and Technology Corporation (JST), Kanagawa 213-0012, Japan
3Joint Research Center for Atom Technology (JRCAT), Tsukuba 305-0046, Japan

Received 10 March 2000; published in the issue dated 28 August 2000

Ultrafast spin dynamics in ferromagnetic half-metallic compound Sr2FeMoO6 is investigated by pump-probe measurements of the magneto-optical Kerr effect. The half-metallic nature of this material gives rise to anomalous thermal insulation between spins and electrons and allows us to pursue the spin dynamics from a few to several hundred picoseconds after the optical excitation. The optically detected magnetization dynamics clearly shows the crossover from microscopic photoinduced demagnetization to macroscopic critical behavior with universal power law divergence of relaxation time for a wide dynamical critical region.

© 2000 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.85.1986
DOI:
10.1103/PhysRevLett.85.1986
PACS:
75.40.Gb, 71.27.+a, 78.20.Ls, 78.47.+p

*Author to whom correspondence should be addressed. Electronic address: gonokami@ap.t.u-tokyo.ac.jp