Phys. Rev. Lett. 86, 2758–2761 (2001)Observation of Triplet Doubly Excited States in Single Photon Excitation from Ground State HeliumReceived 25 October 2000; published in the issue dated 26 March 2001 We have observed, for the first time, LS-forbidden triplet doubly excited states, in single photon excitation of ground state helium, below the second ionization threshold. These states are identified as 3Do and 3Po and their excitation is due to spin-orbit interaction that mixes them with the optically allowed 1Po states. This observation is possible due to the very high efficiency in detecting metastable atoms created after the fluorescence decay of the doubly excited states, and the new capabilities of third generation synchrotron vacuum ultraviolet sources with high resolution beam lines. © 2001 The American Physical Society URL:
http://link.aps.org/doi/10.1103/PhysRevLett.86.2758
DOI:
10.1103/PhysRevLett.86.2758
PACS:
32.80.Dz, 32.50.+d, 32.80.Fb
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