corner
corner

Phys. Rev. Lett. 88, 077204 (2002) [4 pages]

First-Order Transition in the Spin Dynamics of Geometrically Frustrated Yb2Ti2O7

Download: PDF (283 kB) Buy this article Export: BibTeX or EndNote (RIS)

J. A. Hodges1, P. Bonville1, A. Forget1, A. Yaouanc2, P. Dalmas de Réotier2, G. André3, M. Rams4, K. Królas4, C. Ritter5, P. C. M. Gubbens6, C. T. Kaiser6, P. J. C. King7, and C. Baines8
1CEA-Saclay, DRECAM-SPEC, 91191 Gif-sur-Yvette, France
2CEA-Grenoble, DRFMC-SPSMS, 38054 Grenoble, France
3Laboratoire Léon Brillouin, CEA-CNRS, 91191 Gif-sur-Yvette, France
4Institute of Physics, Jagiellonian University, Kraków, Poland
5Institute Laue-Langevin, Grenoble, France
6Interfacultair Reactor Instituut, TU-Delft, 2629 JB Delft, The Netherlands
7Rutherford Appleton Laboratory, Chilton, OX11 0QX, United Kingdom
8Laboratory for Muon Spectroscopy, Paul Scherrer Institute, 5232 Villigen-PSI, Switzerland

Received 4 September 2001; published 1 February 2002

Using neutron diffraction, 170Yb Mössbauer and muon spin relaxation spectroscopies, we have examined the pyrochlore Yb2Ti2O7, where the Yb3+S = 1/2 ground state has planar anisotropy. Below 0.24K, the temperature of the known specific-heat λ transition, there is no long range magnetic order. We show that the transition corresponds to a first-order change in the fluctuation rate of the Yb3+ spins. Above the transition temperature, the rate, in the GHz range, follows a thermal excitation law, whereas below, the rate, in the MHz range, is temperature independent, indicative of a quantum fluctuation regime.

© 2002 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.88.077204
DOI:
10.1103/PhysRevLett.88.077204
PACS:
75.40.-s, 75.25.+z, 76.75.+i, 76.80.+y