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Phys. Rev. Lett. 89, 035002 (2002) [4 pages]

White-Light Nanosource with Directional Emission

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Catherine Favre1, Véronique Boutou1, Steven C. Hill2, Wiebke Zimmer3, Marcel Krenz3, Hendrik Lambrecht1, Jin Yu1, Richard K. Chang4, Ludger Woeste3, and Jean-Pierre Wolf1
1Laboratoire de Spectrométrie Ionique et Moléculaire (UMR5579), Université Lyon 1, 69622 Villeurbanne Cedex, France
2Army Research Laboratory, 2800 Powder Mill Road, Adelphi, Maryland 20783-1197
3Instiut fuer Experimentalphysik, Freie Universitaet Berlin, Arnimallee 14, 10195 Berlin, Germany
4Department of Applied Physics, Yale University, New Haven, Connecticut 06520-8284

Received 27 November 2001; published 26 June 2002

See accompanying Physics Focus

We report the first observation of white-light emission from femtosecond laser-induced plasma in a water droplet. Such emission is not observed with water in a cell. The microdroplet acts as a lens, focusing the incident light to nanosized regions within itself and directing the emission from these regions primarily back toward the laser source. This focusing increases the intensity so that multiphoton ionization generates plasma and causes it to reach the critical density during the initial part of the pulse, enabling the rest of the pulse to heat the plasma enough to emit in the visible.

© 2002 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.89.035002
DOI:
10.1103/PhysRevLett.89.035002
PACS:
52.50.Jm, 42.65.-k, 42.68.Jg