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Phys. Rev. Lett. 89, 075508 (2002) [4 pages]

How Well Do We Know Atomic Motions of Simple Liquids?

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C. Cabrillo1,2, F. J. Bermejo1,2, M. Alvarez2,*, P. Verkerk3,†, A. Maira-Vidal2, S. M. Bennington4, and D. Martín4
1Department of Electricity and Electronics, University Basque Country, P.O. Box 644, E-48080 Bilbao, Spain
2Consejo Superior de Investigaciones Científicas, Serrano 119-123, E-28006 Madrid, Spain
3Interfacultair Reactor Instituut, Technische Universiteit Delft, 2629 JB Delft, The Netherlands
4Rutherford Appleton Laboratory, Chilton, Didcot, Oxon Ox11 0QX, United Kingdom

Received 25 March 2002; published 30 July 2002

Microscopic motions in molten potassium spanning three frequency decades are studied by neutron-scattering techniques. These comprise well-defined density oscillations and stochastic particle rearrangements and both are modeled on microscopic grounds. While vibratory motions are shown to share characteristics with those of their parent crystals, dynamic correlations between a diffusing particle and its neighbors can be accounted for only semiquantitatively.

© 2002 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.89.075508
DOI:
10.1103/PhysRevLett.89.075508
PACS:
61.25.Mv, 61.12.–q, 62.30.+d

*Deceased.

Deceased.