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Phys. Rev. Lett. 90, 128302 (2003) [4 pages]

Pattern of Reaction Diffusion Fronts in Laminar Flows

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M. Leconte, J. Martin, N. Rakotomalala, and D. Salin
Laboratoire Fluides Automatique et Systèmes Thermiques, Universités Pierre et Marie Curie and Paris Sud, C.N.R.S. (UMR 7608) Bâtiment 502, Campus Universitaire, 91405 Orsay Cedex, France

Received 10 October 2002; published 27 March 2003

Autocatalytic reaction between reacted and unreacted species may propagate as solitary waves, namely, at a constant front velocity and with a stationary concentration profile, resulting from a balance between molecular diffusion and chemical reaction. The effect of advective flow on the autocatalytic reaction between iodate and arsenous acid in cylindrical tubes and Hele-Shaw cells is analyzed experimentally and numerically using lattice Bhatnagar-Gross-Krook simulations. We do observe the existence of solitary waves with concentration profiles exhibiting a cusp and we delineate the eikonal and mixing regimes recently predicted.

© 2003 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.90.128302
DOI:
10.1103/PhysRevLett.90.128302
PACS:
82.40.Ck, 47.54.+r, 47.70.Fw