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Phys. Rev. Lett. 90, 133902 (2003) [4 pages]

Two-Photon Ionization of He through a Superposition of Higher Harmonics

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N. A. Papadogiannis1,2, L. A. A. Nikolopoulos1, and D. Charalambidis1,2
1Foundation for Research and Technology-Hellas, Institute of Electronic Structure & Laser, P.O. Box 1527, GR-711 10 Heraklion (Crete), Greece
2University of Crete, Heraklion (Crete), Greece

G. D. Tsakiris, P. Tzallas, and K. Witte
Max Planck Institut für Quantenoptik, D-85748 Garching, Germany

Received 3 July 2002; published 4 April 2003

We present experimental results and theoretical analysis of two-photon ionization of He by a superposition of the 7th to the 13th harmonic of a Ti:sapphire laser. Solving the time-dependent Schrödinger equation for He in a coherent polychromatic field, the He+ yield is calculated. From this yield the number of He+ ions produced has been estimated and found in reasonable agreement with its measured value. The present results establish the feasibility of a second-order autocorrelation measurement of superposition of harmonics, and thus they represent the precursor towards the direct temporal characterization of attosecond pulse trains.

© 2003 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.90.133902
DOI:
10.1103/PhysRevLett.90.133902
PACS:
42.65.Ky, 32.80.Rm