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Phys. Rev. Lett. 90, 223001 (2003) [4 pages]

Switched Wave Packets: A Route to Nonperturbative Quantum Control

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Jonathan G. Underwood1, Michael Spanner1,2, Misha Yu. Ivanov1, Jeff Mottershead1, Benjamin J. Sussman1,3, and Albert Stolow1,3,*
1Steacie Institute for Molecular Sciences, National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario, Canada K1A 0R6
2Department of Physics, University of Waterloo, Waterloo, Ontario, Canada N2L 3G1
3Department of Physics, Queen’s University, Kingston, Ontario, Canada K7L 3N6

Received 19 February 2003; published 4 June 2003

The dynamic Stark effect due to a strong nonresonant but nonionizing laser field provides a route to quantum control via the creation of novel superposition states. We consider the creation of a field-free “switched” wave packet through adiabatic turn-on and sudden turn-off of a strong dynamic Stark interaction. There are two limiting cases for such wave packets. The first is a Raman-type coupling, illustrated by the creation of field-free molecular axis alignment. An experimental demonstration is given. The second case is that of dipole-type coupling, illustrated by the creation of charge localization in an array of quantum wells.

© 2003 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.90.223001
DOI:
10.1103/PhysRevLett.90.223001
PACS:
32.80.Qk, 42.50.Hz

*Electronic address: albert.stolow@nrc.ca