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Phys. Rev. Lett. 90, 257202 (2003) [4 pages]

Magnetic Field Induced Sign Reversal of the Anomalous Hall Effect in a Pyrochlore Ferromagnet Nd2Mo2O7: Evidence for a Spin Chirality Mechanism

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Y. Taguchi1,2, T. Sasaki1, S. Awaji1, Y. Iwasa1, T. Tayama3, T. Sakakibara3, S. Iguchi2, T. Ito4, and Y. Tokura2,4,5
1Institute for Materials Research, Tohoku University, Sendai 980-8577, Japan
2Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan
3Institute for Solid State Physics, University of Tokyo, Kashiwa 277-8581, Japan
4Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba 305-8562, Japan
5Spin Superstructure Project (SSS), ERATO, Japan Science and Technology Corporation (JST), Tsukuba 305-8562, Japan

Received 24 January 2003; published 25 June 2003

The anisotropic Hall effect and magnetization have been investigated for single crystals of Nd2Mo2O7 under high magnetic fields up to 27 T and at low temperatures down to 50 mK. The magnetization curves indicate that the Nd moments with strong Ising anisotropy are coupled antiferromagnetically with the Mo spins and show field-induced flipping on the respective sites. The Hall resistivity changes its sign with increasing field applied along the [111] direction, while it monotonously approaches zero with the field applied along the [100] or [110] direction. This behavior is in accord with the prediction by the Berry phase theory and is interpreted in terms of the field-induced reversal of spin chirality on the pyrochlore lattice.

© 2003 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.90.257202
DOI:
10.1103/PhysRevLett.90.257202
PACS:
75.47.–m, 75.30.Mb, 75.50.Cc