corner
corner

Phys. Rev. Lett. 93, 147402 (2004) [4 pages]

Quantum Mechanical Single-Gold-Nanocluster Electroluminescent Light Source at Room Temperature

Download: PDF (374 kB) Buy this article Export: BibTeX or EndNote (RIS)

Jose I. Gonzalez1, Tae-Hee Lee1, Michael D. Barnes2, Yasuko Antoku1, and Robert M. Dickson1,3,*
1School of Chemistry and Biochemistry, Georgia Institute of Technology, Atlanta, Georgia 30332-0400, USA
2Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee, USA
3Center for Advanced Research in Optical Microscopy, Georgia Institute of Technology, Atlanta, Georgia 30332-0400, USA

See Also: Publisher's Note

Received 5 May 2004; published 27 September 2004; publisher error corrected 4 October 2004

Electrically contacted gold-nanocluster arrays formed within electromigration-induced break junctions exhibit bright, field-dependent electroluminescence in the near infrared (650–800 nm). Intensity autocorrelation of spatially isolated individual nanocluster emission driven at high electrical frequency (fac=∼200  MHz) reveals antibunched electroluminescence at room temperature. These results demonstrate the single quantum nature of several-atom gold molecules and suggest their use as room-temperature electrically driven single-photon sources.

© 2004 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.93.147402
DOI:
10.1103/PhysRevLett.93.147402
PACS:
78.60.Fi, 42.50.–p, 78.67.Bf, 85.60.Jb

*To whom correspondence should be addressed. dickson@chemistry.gatech.edu

See Also

Publisher's Note: Jose I. Gonzalez, Tae-Hee Lee, Michael D. Barnes, Yasuko Antoku, and Robert M. Dickson, Publisher's Note: Quantum Mechanical Single-Gold-Nanocluster Electroluminescent Light Source at Room Temperature [Phys. Rev. Lett. 93, 147402 (2004)], Phys. Rev. Lett. 93, 159903 (2004).