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Phys. Rev. Lett. 93, 193001 (2004) [4 pages]

Photoexcitation of He- Hollow-Ion Resonances: Observation of the 2s2p24P State

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R. C. Bilodeau1,2, J. D. Bozek2, A. Aguilar2,3, G. D. Ackerman2, G. Turri1,2, and N. Berrah1
1Western Michigan University, Physics Department, Kalamazoo, Michigan 49008-5151, USA
2Lawrence Berkeley National Laboratory, Advanced Light Source, Berkeley, California 94720, USA
3University of Nevada, Department of Physics, Reno, Nevada 89557-0058, USA

Received 26 April 2004; published 4 November 2004

Highly correlated states are studied in He-, a fundamental 3-electron system and prototypical negative ion. The 2s2p24P state is observed for the first time. This state is detected in a resonant simultaneous double-Auger decay of unprecedented strength. In addition, the first measurements of photodetachment cross sections, positions, widths, and shapes of triply excited resonances in He- are reported. These measurements provide a sensitive test for several sophisticated ab initio calculations, and indicate differences in the position and shape of some structures.

© 2004 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.93.193001
DOI:
10.1103/PhysRevLett.93.193001
PACS:
32.80.Hd, 32.80.Gc