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Phys. Rev. Lett. 93, 213003 (2004) [4 pages]

Absolute Ionization Rates of Multielectron Transition Metal Atoms in Strong Infrared Laser Fields

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Marc Smits1, C. A. de Lange1, Albert Stolow2,*, and D. M. Rayner2,†
1Department of Physics and Astronomy, Vrije Universiteit Amsterdam, Netherlands
2Steacie Institute for Molecular Sciences, National Research Council Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6 Canada

Received 31 May 2004; published 15 November 2004

We report on nonresonant strong field ionization of the multielectron transition metal atoms V, Nb, Ta, Ni, and Pd. Operating in the adiabatic regime (λ=1.5  μm), we quantitatively determined both (i) the first charge state saturation intensities and (ii) the absolute ionization rates for intensities ranging from threshold up to 3×1014  W/cm2. We observed a dramatic suppression of ionization relative to single active electron approximation expectations. We suggest that this derives from dynamic polarization or screening effects within the multielectron atom, stressing a need for many-body theories of strong field ionization.

© 2004 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.93.213003
DOI:
10.1103/PhysRevLett.93.213003
PACS:
32.80.Rm, 42.50.Hz

*Electronic address: albert.stolow@nrc-cnrc.gc.ca

Electronic address: david.rayner@nrc-cnrc.gc.ca