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Phys. Rev. Lett. 94, 036405 (2005) [4 pages]

Mott Phase at the Surface of 1T-TaSe2 Observed by Scanning Tunneling Microscopy

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Stefano Colonna1, Fabio Ronci1, Antonio Cricenti1,2, Luca Perfetti3, Helmuth Berger4, and Marco Grioni3
1CNR Istituto di Struttura della Materia, Via Fosso del Cavaliere, 100, 00133 Roma Italy
2Department of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235-1807, USA
3Institut de Physique des Nanostructures, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland
4Institut de Physique de la Matiere Complexe, Ecole Polytechnique Federale de Lausanne, CH-1015 Lausanne, Switzerland

Received 5 July 2004; published 25 January 2005

In this Letter we report the observation, by scanning tunneling microscopy, of a Mott metal to insulator transition at the surface of 1T-TaSe2. Our spectroscopic data compare considerably well with previous angle-resolved photoemission spectroscopy measurements and confirm the presence of a large hysteresis related to a first order process. The local character of the tunneling spectroscopy technique allows a direct visualization of the surface symmetry and provides spectroscopic measurements on the defect-free region of the sample. It follows that the electronic localization is driven purely by the enhancement of the charge density wave amplitude which drives a bandwidth controlled metal-insulator transition.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.94.036405
DOI:
10.1103/PhysRevLett.94.036405
PACS:
71.30.+h, 68.37.Ef