Phys. Rev. Lett. 95, 023001 (2005) [4 pages]Direct Frequency Comb Measurements of Absolute Optical Frequencies and Population Transfer DynamicsReceived 12 March 2005; published 6 July 2005 A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled 87Rb atoms. Absolute atomic transition frequencies, such as the 5S1/2 F=2→7S1/2 F′′=2 two-photon resonance measured at 788 794 768 921 (44) kHz, are determined without a priori knowledge about their values. Detailed dynamics of population transfer driven by a sequence of pulses are uncovered and taken into account for the measurement of the 5P states via resonantly enhanced two-photon transitions. © 2005 The American Physical Society URL:
http://link.aps.org/doi/10.1103/PhysRevLett.95.023001
DOI:
10.1103/PhysRevLett.95.023001
PACS:
32.80.−t, 32.80.Qk, 39.25.+k, 39.30.+w
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