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Phys. Rev. Lett. 95, 237602 (2005) [4 pages]

Polarization Relaxation Induced by a Depolarization Field in Ultrathin Ferroelectric BaTiO3 Capacitors

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D. J. Kim1, J. Y. Jo1, Y. S. Kim1, Y. J. Chang1, J. S. Lee1, Jong-Gul Yoon2, T. K. Song3,*, and T. W. Noh1
1ReCOE and School of Physics, Seoul National University, Seoul 151-747, Korea
2Department of Physics, University of Suwon, Kyunggi-do 445-743, Korea
3Department of Ceramic Science and Engineering, Changwon National University, Changwon, Kyungnam 641-773, Korea

Received 21 June 2005; published 1 December 2005

Time-dependent polarization relaxation behavior induced by a depolarization field Ed was investigated on high-quality ultrathin SrRuO3/BaTiO3/SrRuO3 capacitors. The Ed values were determined experimentally from an applied external field to stop the net polarization relaxation. These values agree with those from the electrostatic calculations, demonstrating that a large Ed inside the ultrathin ferroelectric layer could cause severe polarization relaxation. For numerous ferroelectric devices of capacitor configuration, this effect will set a stricter size limit than the critical thickness issue.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.95.237602
DOI:
10.1103/PhysRevLett.95.237602
PACS:
77.22.Ej, 77.22.Gm, 77.55.+f, 77.80.Dj

*Electronic mail: tksong@changwon.ac.kr