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Phys. Rev. Lett. 96, 177002 (2006) [4 pages]

Effect of Irradiation-Induced Disorder on the Conductivity and Critical Temperature of the Organic Superconductor κ-(BEDT-TTF)2Cu(SCN)2

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James G. Analytis1, Arzhang Ardavan1, Stephen J. Blundell1, Robin L. Owen2, Elspeth F. Garman2, Chris Jeynes3, and Ben J. Powell4
1Department of Physics, Clarendon Laboratory, University of Oxford, Parks Road, Oxford OX1 3PU, United Kingdom
2Department of Biochemistry, University of Oxford, South Parks Road, Oxford OX1 3QU, United Kingdom
3University of Surrey Ion Beam Centre, Guildford GU2 7XH, United Kingdom
4Department of Physics, University of Queensland, Brisbane, Queensland 4072, Australia

Received 1 December 2005; published 3 May 2006

We have introduced defects into clean samples of the organic superconductor κ-(BEDT- TTF)2Cu(SCN)2 in order to determine their effect on the temperature dependence of the interlayer conductivity σ and the critical temperature Tc. We find a violation of Matthiessen’s rule that can be explained by a model of σ involving a defect-assisted interlayer channel which acts in parallel with the bandlike conductivity. We observe an unusual dependence of Tc on residual resistivity, inconsistent with the generalized Abrikosov-Gor’kov theory for an order parameter with a single component, providing an important constraint on models of the superconductivity in this material.

© 2006 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.96.177002
DOI:
10.1103/PhysRevLett.96.177002
PACS:
74.70.Kn, 74.25.Fy, 74.62.Dh