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Phys. Rev. Lett. 96, 223902 (2006) [4 pages]

Role of Many-Electron Dynamics in High Harmonic Generation

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Ariel Gordon1,*, Franz X. Kärtner1, Nina Rohringer2, and Robin Santra2
1Department of Electrical Engineering and Computer Science and Research Laboratory of Electronics, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, USA
2Argonne National Laboratory, Argonne, Illinois 60439, USA

Received 30 January 2006; revised 3 May 2006; published 6 June 2006

High harmonic generation (HHG) in many-electron atoms is studied theoretically. The breakdown of the frozen-core single active electron approximation is demonstrated, as it predicts roughly the same radiation amplitude in all noble gases. This is in contradiction with experiments, where heavier noble gases are known to emit much stronger HHG radiation than lighter ones. This experimental behavior of the noble gases can be qualitatively reproduced when many-electron dynamics, within a simple approximation, is taken into account.

© 2006 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.96.223902
DOI:
10.1103/PhysRevLett.96.223902
PACS:
42.65.Ky, 32.80.Rm

*Electronic address: gariel@mit.edu