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Phys. Rev. Lett. 97, 055504 (2006) [4 pages]

Universal Features of Terahertz Absorption in Disordered Materials

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S. N. Taraskin1,2,*, S. I. Simdyankin2, S. R. Elliott2, J. R. Neilson2,3, and T. Lo4
1St. Catharine’s College, Trumpington Street, Cambridge CB2 1RL, United Kingdom
2Department of Chemistry, University of Cambridge, Cambridge CB2 1EW, United Kingdom
3Department of Materials Science and Engineering, Lehigh University, Bethlehem, Pennsylvania 18015, USA
4Teraview Ltd., Platinum Building, St. John’s Innovation Park, Cambridge CB4 OW5, United Kingdom

Received 10 March 2006; published 2 August 2006

Using an analytical theory, experimental terahertz time-domain spectroscopy data, and numerical evidence, we demonstrate that the frequency dependence of the absorption coupling coefficient between far-infrared photons and atomic vibrations in disordered materials has the universal functional form, C(ω)=A+Bω2, where the material-specific constants A and B are related to the distributions of fluctuating charges obeying global and local charge neutrality, respectively.

© 2006 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.97.055504
DOI:
10.1103/PhysRevLett.97.055504
PACS:
63.50.+x, 61.43.Fs, 78.30.Ly

*Electronic address: snt1000@cam.ac.uk