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Phys. Rev. Lett. 98, 256804 (2007) [4 pages]

Berry-Phase Blockade in Single-Molecule Magnets

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Gabriel González1,2 and Michael N. Leuenberger1,2,*
1NanoScience Technology Center, University of Central Florida, Orlando, Florida 32826, USA
2Department of Physics, University of Central Florida, Orlando, Florida 32816, USA

Received 24 October 2006; published 20 June 2007

We formulate the problem of electron transport through a single-molecule magnet (SMM) in the Coulomb blockade regime taking into account topological interference effects for the tunneling of the large spin of a SMM. The interference originates from spin Berry phases associated with different tunneling paths. We show that, in the case of incoherent spin states, it is essential to place the SMM between oppositely spin-polarized source and drain leads in order to detect the spin tunneling in the stationary current, which exhibits topological zeros as a function of the transverse magnetic field.

© 2007 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevLett.98.256804
DOI:
10.1103/PhysRevLett.98.256804
PACS:
73.23.Hk, 03.65.Vf, 75.45.+j, 75.50.Xx

*mleuenbe@mail.ucf.edu