Time-resolved optical reflectivity of the electron-doped Nd2-xCexCuO4 + \delta cuprate superconductor: Evidence for an interplay between competing orders

Accepted

We use pump-probe spectroscopy to measure the photoinduced reflectivity $\Delta R$ of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_{x}$CuO$_{4+\delta}$ at a value of $x$ near optimal doping, as a function of time, temperature, and laser fluence. We observe the onset of a negative $\Delta R$ signal at $T^{*} \approx 75$~K, above the superconducting transition temperature, $T_{c}$, of 23 K. The relatively slow decay of $\Delta R$, compared to the analogous signal in hole doped compounds, allows us to resolve time-temperature scaling consistent with critical fluctuations. A positive $\Delta R$ signal onsets at $T_{c}$ that we associate with superconducting order. We find that the two signals are strongly coupled below $T_{c}$, in a manner that suggests a repulsive interaction between superconductivity and another fluctuating order.