Unanticipated proximity behavior in ferromagnet-superconductor heterostructures with controlled magnetic noncollinearity

Accepted

Magnetization non-collinearity in ferromagnet (F)/superconductor (S) heterostructures is expected to enhance the superconducting transition temperature (Tc) according to the domainwall superconductivity theory, or to suppress Tc when spin-triplet Cooper pairs are explicitly considered. We study the proximity effect in F/S structures where the F-layer is a Sm-Co/Py exchange-spring bilayer and the S-layer is Nb. The exchange-spring contains a single, controllable and quantifiable domain wall in the Py layer. We observe an enhancement of superconductivity that is non-monotonic as the Py domain wall is increasingly twisted via rotating a magnetic field, different from theoretical predictions. We have excluded magnetic fields and vortex motion as the source of the non-monotonic behavior. This unanticipated proximity behavior suggests that new physics is yet to be captured in the theoretical treatments of F/S systems containing non-collinear magnetization.